Resolving Crackling, Throttling, and "Ultmate Performance Option" in Lenovo Thinkpad P16 (Gen 2)

It should be .ps1 not .psi

About the execution policy: right click on the SetSafeUltimate.ps1:

In the popup menu click ‘properties’. Probably at the bottom there’s a message about the file being blocked, because it’s from the internet. Remove the block and try again.

Maybe post a screenshot in this thread of the powershell window with the command executed (or having failed to execute)